The interest in multiferroic materials has increased in the last few
years due to the fundamental physics of strong interaction between
ferroelectric and magnetic orders, as well as for the promise of novel
applications in future electronics. From powerful symmetry arguments
and with modeling of the microscopic coupling mechanism, these efforts
have led to the discovery of a vast set of multiferroic compounds. An
important recent step in this regard was the discovery of a new kind of
magnetic excitation that couples strongly to light by acquiring
electric dipole activity from the infrared active phonons, called
electromagnon, which is a hybrid excitation of magnon and phonon
character. These discoveries have highlighted the importance of the
dynamical aspects of the magnetoelectric coupling.
Based on measurements of the electrodynamic spectra as function of
temperature and magnetic field in multiferroic RMnO
3 and RMn
2O
5,
a model of the electromagnon response is developed. This results
in the direct excitation of a Brillouin zone boundary magnon by the
electric field of the electromagnetic wave, as opposed to the usual
magnetic resonance which is the zone center magnon excited by the
magnetic field of light. These results demonstrate that the symmetric
exchange interaction is responsible for all the observed dynamic
magnetoelectric effects, and opens a new avenue for studying
multiferroic and frustrated magnets.